How can I adjust the width percentage or pixel parameter for each layout?

Can someone take a minute or two to record a quick screencast on how to update the .css or .less files at a site and/or group level, illustrating where to go and how you would change/update these files?

For example... let's say that I wanted to use this layout:

Lets also assume the default setting is 75% on the left column and 25% on the right column. How could I change the right column to be 310px? What about if I wanted that right column to be 35% of the page?

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